Chinese Journal of Oceanology and Limnology
Vol. 27 No. 2, P. 266-276, 2009
DOI: 10.1007/s00343-009-9118-y
The impact of physical processes on pollutant transport in
Hangzhou Bay*,,**
LI Ning, MAO Zhihua, ZHANG Qinghe School of Civil Engineering, Tianjin University; Key Laboratory of Harbor and Ocean Engineering, Ministry of Education of
China, Tianjin 300072, China
State Key Laboratory of Satellite Ocean Environment Dynamic, Second Institution of Oceanography, State Oceanic
Administration, Hangzhou 310012, China
Received May 9, 2008; revision accepted Dec. 1, 2008
Abstract A Lagrangian tracer model is set up for Hangzhou Bay based on Coupled Hydrodynamical
Ecological model for Regional Shelf Sea (COHERENS). The study area is divided into eight subdomains
to identify the dominant physical processes, and the studied periods are March (the dry season) and July
(the wet season). The model performance has been first verified by sea-surface elevation and tidal current
observations at several stations. Eight tracer experiments are designed and Lagrangian particle tracking is
simulated to examine the impact of physical processes (tide, wind and river runoff) on the transport of
passive tracer released within the surface layer. Numerical simulations and analysis indicate that: (1) wind
does not change the tracer distribution after 30 days except for those released from the south area of the
bay during the wet season; (2) the tide and the Qiantang River runoff are important for particle transport
in the head area of the bay; (3) the Changjiang River runoff affects the tracer transport at the mouth of the
bay, and its impact is smaller in the dry season than in the wet season.
Keyword: Hangzhou Bay; pollutant transport; COHERENS; tracer experime
1 INTRODUCTION Both the report of marine environment in Zhejiang
Province in 2007 and the report of Chinese marine
Hangzhou Bay is located in the northern Zhejiang
environmental quality in 2007 point out that the
Province, with water depth of 8 10 m. It is the outer
environmental quality of the most area in Hangzhou
part of the Qiantang River Estuary, adjacent to the
Bay is worse than Grade IV. Wetlands are decreasing
East China Sea and with the Zhoushan Archipelago
at an annual rate of approximately 5%, and marine
located in the southeast of the embayment (Fig.1).
biodiversity keeps declining. About 96.7% of the
The bay is affected by both the river runoff and the
sewage outlets being monitored discharge pollutants
tide. The tidal current is strong, and the mean tidal
in excess of the limits set by the national standards.
range increases progressively from the mouth to the
Field investigation in the fishery waters near the
head of the bay. At the Ganpu station located at the
Yangtze Estuary and Hangzhou Bay in the months of
head of the bay, the mean tidal range is 5.54 m and
May and August from 2000 to 2002 shows that the
the maximum tidal range can reach 8.93 m. The tidal
pollution index of Cu is 5.84 and 4.28 for Zn, and the
currents within the bay are mainly rectilinear, with
comprehensive index of multifactors is 1.99, which is
maximum velocities above 2 m/s near the mouth and
far beyond the serious pollution level of 1.67 (Shen et
greater than 4 m/s in the head areas (Zhou and Gao,
al., 2003). The data obtained during rainy seasons of
2004). The bay is also affected by two large rivers,
recent years show that the nitrogen and phosphorus
the Changjiang River and the Qiantang River, with
concentrations in the bay exceed their standard
mean river discharges of about 9 529 108 m3 (Chen
values severely. For the structure of nutrients, the
et al., 2007) and 373 108 m3 (Ni et al., 2003),
respectively. The prevailing wind direction is SE-S
* Supported by the Natural Science Foundation of China (No.40576080);
in summer, and N-NE in winter (Wang and Cheng,
National High Technology Research and Development Program of China
1995), and the average wind speed is 3 m/s in (863 Program, No. 2007AA12Z182)
summer and 6 m/s in winter (Zhu et al., 2004). ** Corresponding author: *********@***.***
267
No.2 LI et al.: The impact of physical processes on pollutant transport in Hangzhou Bay
river discharge on driving pollution transport in
different areas of the bay. So, the aim of the present
study is to set up a Lagrangian tracer model based on
COHERENS (Coupled Hydrodynamical Ecological
Model for Regional Shelf Seas) to simulate the
impact of various physical processes (wind, tide, and
river runoff) on the pollutant transport in different
areas of the bay in the wet and dry seasons.
The paper is organized as follows. Section 2 gives
a brief description of the numerical model, followed
by model validation in section 3. Tracer experiments
and results are described in section 4 and 5. Sections
6 and 7 provide discussions and conclusions,
respectively.
Fig.1 Sea floor topography of the study area, five tide gauges
(square) and two current stations (triangle)
2 NUMERICAL MODELS
ratio of nitrogen to phosphorus is as high as 405
2.1 Hydrodynamic model
(Wang et al., 2006). Side source and disorder
drainage of pollution material have obviously
COHERENS is a three-dimensional hydrodynamic
affected water quality of Hangzhou Bay (Zhang et al.,
multi-purpose model for coastal and shelf seas. The
2002). Clearly, the water quality has been in a state of
model was selected for the investigation of
severe eutrophication.
Hangzhou Bay because it is an integrated model,
In recent years, many researchers have studied the
which couples the modules that simulate physical
pollutant transport in the bay using different approaches.
and biological processes, sediments and contaminant
Li and Sun (1995) used a 3-D hydrodynamic numerical
transport and resolve mesoscale to seasonal scale
model on -coordinate to simulate the tide-induced
processes (Luyten et al., 1999). The user has the
Euler residual currents and Lagrangian residual
choice of several state-of-the-art advection schemes
currents, residual drifts and tracks of water particles.
for momentum and scalars, and the model allows for
Wang and Cheng (1995) investigated the temporal
various parameterisations of turbulent motion
and spatial variations of the flow field in Hangzhou
including a variety of turbulence closure schemes.
Bay and the pollution risk caused by oil spill accident
The model is freely available and well documented,
under different weather conditions. Shi et al. (2000)
and has been widely used in the North Sea and other
and Zhu et al. (2000) simulated the residual current
areas (Umgiesser et al., 2002; Jiang, 2004; Lacroix et
and its effect on mass transport with a 3-D joint
al., 2004; Carafa et al.,2006; Marinov et al.; 2006;
model of Hangzhou Bay and the Yangtze Estuary,
Chen et al., 2007; Ribbe et al., 2008). The model is
considering the impacts of river flow, wind,
based on the Boussinesq approximation and vertical
baroclinic pressure, current of the East China Sea and
hydrostatic equilibrium. The primitive equations for
tide. He (2000) studied pollution transport along the
the three-dimensional mode in the coordinate are
northern coast of Hangzhou Bay in different tidal
phases. Lin et al. (2005) established a 2-D
1 J + 1 ( Ju ) + 1 ( Jv ) + 1 ( Jw ) = 0
hydrodynamic model to get the flow field near the
J t J x1 J x2 J x3
disposal point in Hangzhou Bay and then used the
PLUME model to simulate the dilution ability of a (1)
diffuser. Lin et al. (2008) set up a large scale 3-D
1 J ( Ju) + 1 (Ju2 ) + 1 (Jvu) + 1 ( Jwu) fv =
flow and salinity model and a smaller scale discharge J x1 J x2 J x3
J t
diffuser model to study the high salt effluent
g 1 Pa + Q1 + 1 ( T u ) + 1 (J 11) +
v
discharge and its maximum load control in Hangzhou 0 x1
x1 J x3 J x3 J x1
Bay. With water pollution control being mainly 1 (J )
concentrated on industrial point sources (Chau and J x2 21
Jiang, 2002; Lale, 2001), there are few studies of side
(2)
source pollution of the bay. What is more, even less
attention has been paid to the role of tide, wind, and
268 CHIN. J. OCEANOL. LIMNOL., 27(2), 2009 Vol.27
1 J (Jv) + 1 (Juv) + 1 (Jv2) + 1 (Jwv) + fu = Lagrangian tracer method for constructing trace of a
J x1 J x21 J x3
J t single particle is suitable to simulate the pollution
g 1 P + Q2 + 1 (
vT v 1 trajectory and to solve water pollution problems, so it
(J ) +
)+
a
x2 0 x2 J x3 J x3 J x1 12
is widely applied to trace pollutant particles
1 (J ) (Tartinville et al., 1997; Cetina et al., 2000; Kraines
J x21 22
et al., 2001; Siegel et al., 2003; Wong et al., 2004;
Chen et al., 2007). The present work focuses mainly
(3)
on the COHERENS physical and Lagrangian
1 qd = b ( 4)
modules to simulate the advective-diffusive transport
J x3
of contaminants in the bay. The primitive equation is
1 ( JC) + 1 ( JuC) + 1 ( JvC) + 1 ( JwC) =
1 J ( JT ) + 1 ( JuT ) + 1 ( JvT ) +
J x1 J x1 J x2 J x3
J x1 J x2
J t
1 ( T C ) + 1 ( T C ) + 1 (J C ) +
( T T ) +
( Jw ) = 1 I + 1
1 J x3 J x3 J x3 J x3 J x1 H x
J 0 c P x3 J
x3 x3 J x3
J 1
1 ( J C )
( J T ) + 1 ( J T )
1
J x2 H x
2
H
x1 J x2 x2
J H
(7)
(5)
where C represents a number of particles, each
1 J ( J S ) + 1 ( JuS ) + 1 ( JvS ) +
having a certain amount of load and with an initial
J x1 J x2
J t
position. Each particle has a specific label, which
T S
1 ( Jw S ) = 1 +
allows for the tracing of the individual particle or
J x3 J x3 J x 3
isolating the distribution of particles. The transport of
1 ( J S ) + 1 ( J S )
particles is determined by the horizontal and vertical
J x1 H x J x2 H x
2
1
advections and turbulent diffusions. The vertical and
(6) horizontal diffusions of these suspended particles are
where J = x3 / x3 represents the ratio of a unit determined by using a random walk method, which is
the most accurate and capable of handling
length in the physical to a unit length in the
complexities in the flow field (Kraines et al. 2006).
transformed space; ( x1, x2, x3 ) represent the three
directions in coordinate; ( u, v, w ) are the
2.2 Numerical simulation
components of the current; T denotes the
temperature; S the salinity; f the Coriolis frequency; Previous investigations indicated that pollutant
transport in Hangzhou Bay is interconnected to
g the acceleration of gravity; Pa the atmospheric
physical transport in the Yangtze Estuary (Ni et al.,
pressure at the surface; Q1, Q2 the components of
the baroclinic pressure gradient; vT and T the 2003; Lu et al., 2006). Thus, the model domain
includes both Hangzhou Bay and the Yangtze
vertical eddy viscosity and diffusion coefficients;
Estuary, covering the area of 120 124 E;
H the horizontal diffusion coefficient for salinity
and temperature; 0 a reference density; c p the 29.5 32.5 N (Fig.1). To simplify the discussion, the
year has been divided into two seasons, the wet
specific heat of seawater; I solar irradiance;
11, 12, 21, 22 the horizontal components of the season and the dry season, and the study is focused
on two typical months, July in 2005 (in the wet
stress tensor; qd the baroclinic pressure; b the
season) and March in 2006 (in the dry season). In
buoyancy. Eq.1 is the continuity equation, Eqs.2 and
addition, the domain is further divided into 8
3 are the horizontal momentum equations, Eq.4 is the
subdomains (Fig.2). Passive tracers designed to
hydrostatic equation, Eq.5 is the temperature
represent contaminant particles are released in
equation and Eq.6 is the salinity equation. These
surface layers of each subdomain, thus the tracer
equations are discretized on the Arakawa-C grid with
a -coordinate in the vertical direction. The transport trajectories can be simulated separately.
Each particle has been tracked for 1 month or until it
advection of momentum and scalars in the program
leaves the model domain whichever comes first.
apply the Total Variation Diminishing (TVD)
The model includes realistic coastline and
scheme. The horizontal diffusion coefficients are
topography; it is forced by the surface wind stress
implemented the Smagorinsky parameterization. The
and the QSCAT/NCEP Blended Ocean Winds from
well-known mode-splitting technique is employed to
Colorado Research Associates are used as the input
solve the momentum and continuity equations. The
269
No.2 LI et al.: The impact of physical processes on pollutant transport in Hangzhou Bay
winds. In addition, the tidal harmonic constants of the document by Du et al. (2007). Due to the
the four tidal components (K1, O1, M2, and S2) are limitation of space, only part of the verification
specified. The runoff discharge from the Changjiang results are shown below, including the calibration
River is set at 41 000 m3/s in the wet season and results for sea surface elevation modelled by
21 000 m3/s in the dry season. Since the discharge COHERESN and observed at the L huashan and
Shenjiamen tide gauges in July (Fig.3), and current
from the Qiantang River is far less than that from the
velocities (Fig.4) and current directions (Fig.5)
Changjiang River, it was taken as 3.15% of that one
modelled and observed at water surface, 5.6 m below
from the Changjiang River. A rectangular grid is
surface and bottom during July 13 14, 2005. It can
designed to map the domain in 100 100 points with a
be seen that the simulated results agree well with the
resolution of 0.03 in longitude and 0.04 in latitude.
observations. The computational result basically
Ten sigma layers are used in the vertical direction.
expresses the characteristic of the water dynamic
This spatial resolution restricts the model time step to
condition in the domain area.
2.5 s. For horizontal currents, the surface boundary
condition is obtained by specifying the surface stress
4 TRACE EXPERIMENTS
as a function of wind speed components, while the
bottom friction is defined by slip boundary condition. It is well known that the fate of pollutant is
In this case, a vertical uniform bottom stress is determined by the wind, tide and runoff of rivers.
assumed yielding a logarithmic profile for the current Thus, to estimate the influence of the physical factors
and the bottom velocities are evaluated at the grid on pollutant transport in Hangzhou Bay, eight tracer
points nearest to the bottom layer. The bottom drag experiments have been designed with the model
coefficient is expressed as a quadratic function of bed forced by different combinations of these physical
roughness length with a value of 0.002 m which is factors in the wet and dry seasons (Table 1). Two
uniform in space and constant in time. The months, July in 2005 and March in 2006, are
calculation starts with zero values for currents and specified to represent the wet seasons and dry
surface elevation. No special efforts about different seasons, respectively. The wind and the river runoff
model accelerations in order to attain convergence of in these two months are used in the simulation. The
the numerical solution have been made because it tidal harmonic constants of the four tidal components
was found that the model reaches good numerical (K1, O1, M2, and S2) are derived from the atlas of
convergence (Luyten et al., 1999). marine hydrology. Except in E1 and E5, one of these
three physical factors (wind, tide and river runoff) is
eliminated by setting the value of the corresponding
parameter to zero. For example, in E2 and E6, the
river runoff and the wind are considered, while the
tide is disregarded by setting the amplitude of the
four tidal components to zero. The same setting are
performed in E3, E4, E7 and E8, in which the value
of the river runoff or the wind speed is set to zero,
respectively.
5 RESULTS
The trajectories of tracers released from the 8
subdomains were calculated separately, and then
those particles in the eight experiments were further
Fig.2 The eight subdomains in the COHERENS model
binned after 30 days. Fig.6 shows the pollutant
distribution of E1 to E4 in 8 subdomains in the wet
3 VERIFICATION OF THE MODEL
season and Fig.7 shows that of E5 to E8 after 30 days
The model has been verified by observations from in the dry season. Forced by tide, wind and river
the 5 tide Gauges-L huashan, Shenjiamen, Tanhu, runoff (the first column of Fig.6 and Fig.7), the
Zhongjun and Luchaogang (Fig.1) in July, 2005 and particles run southeast, travel around the Zhoushan
in March, 2006, and the mooring stations in C1 from Archipelago, and then escape from the bay. Among
July 13 to July 14 and in C2 from July 6 to July 7 in those particles getting out of the bay, the ones
2005. The mooring station data is digitalized from released from the bay mouth area (S3, S6, S8) take up
270 CHIN. J. OCEANOL. LIMNOL., 27(2), 2009 Vol.27
Fig.3 Sea surface elevation obtained from COHERENS (solid line) and tide gauges observation (dot) form July 1 31, 2005
a. L huashan; b. Shenjiamen
Fig.4 Current velocities obtained from COHERENS (solid line) and observations (dish line) in 30.6 N, 122.25 E from 15:00,
July 13, 2005 to 15:00, July 14, 2005
a. surface; b. 5.6m below surface; c. bottom
taken outside and they are responsible for the
a major portion, while the ones from the middle of the
eutrophication in the bay.
bay (S2, S5, S7) occupy a small potion. No particles
from the inner side of the bay (S1, S4) leave there
5.1 No tidal forcing
after 30 days. Thus it can be concluded that the
If the tidal forcing is not considered, in the wet season
pollutants from the bay head area are difficult to be
271
No.2 LI et al.: The impact of physical processes on pollutant transport in Hangzhou Bay
Fig.5 Current direction obtained from COHERENS (solid line) and observations (dish line) in 30.6 N, 122.25 E from 15:00,
July 13, 2005 to 15:00, July 14, 2005
a. surface; b. 5.6m below surface; c. bottom
Table 1 Eight trace experiments in the COHERENS model with different season and input set
Tracer experiments Season Input Tracer experiments Season Input
E1 Wet River, wind, tide E5 Dry River, wind, tide
E2 Wet River, wind E6 Dry River, wind
E3 Wet River, tide E7 Dry River, tide
E4 wet Tide, wind E8 Dry Tide, wind
(the second column of Fig.6), particles deflect to run particle trajectory in the other subdomains in this
westward in general. The ones released from most season does not change much. In the dry season (the
subdomains of the bay (S1, S2, S4, S5, S7 and S8) third column of Fig.7), the particle transport in the
would advance upstream towards the Qiantang River, whole bay does not vary much compared with E5.
while the ones from S3 and S6 firstly approach the
5.3 No river runoff
south shore, then go around the Zhoushan
If we do not consider the river runoff, in the wet
Archipelago, and finally leave the bay. In the dry
season (the fourth column of Fig.6), the traces of
season (the second line of Fig.7), similar results were
particles released from S2, S3, S6, S8 change
observed for the particles from S1 S6 as in the wet
significantly, and tend to run towards the north and
season, but for the ones from S7 and S8, it is more
northeast, which are different directions when the
easily to get out of the bay than in the wet season
river is considered; Particles from S4, S5 and S7
without the force of tide.
tends to travel upstream towards the Qiantang River.
5.2 No wind In the dry season (the fourth column of Fig.7), the
particle transport is similar to that in the wet season.
If no account is taken of the wind, in the wet
To conclude, the pollutant transport depends on
season (the third column of Fig.6), particles from S4
the tide, wind and river runoff. The influence of these
move much farther towards the southeast, particles
physical factors on the pollutant transport in different
from S5 and S7 advance along the south shore and
subdomains is different. The tide and river runoff are
more particles from S8 get out of the bay. The
272 CHIN. J. OCEANOL. LIMNOL., 27(2), 2009 Vol.27
important dynamic forcing factors, and the wind just Although the extreme sea events would determine
affects the particle transport in a few subdomains in material transport and dynamic balance (Yin et al.,
the wet season. 2007), they do not often occur, so in this paper we
just take the normal wind into consideration.
6 DISCUSSION Generally, wind is the comparatively weak dynamic
factor among these three physical factors. In the wet
The tracer experiments discussed in this study are
season the wind pushes the released particles from S5
focused on the trajectory of the tracers released in
and S7 a short distance off the south shore and pushes
Hangzhou Bay. These tracers represent both
the particles from S8 back to the bay. This is the
dissolved materials and materials released into the
result of the S and SE winds during the wet months
water column by geochemical and biological
which will blow the particles released from the south
processes.
area of the bay towards the north and northwest. In
Depending on the property, tracers can be
the dry season, the pollutant trajectory is not affected
classified into passive tracers, active tracers,
by the wind as shown in Fig.7. The current induced
dynamic active tracers, or interactive tracers. As a
by the wind is strong at the surface, and can reach
first step towards the simulation of the
more than 20 cm/s (Zhu et al., 2000), but this current
transportation of many kinds of pollutants, our goal
decreases quickly with depth. Nearly 80% of the
in this study is confined to the water-borne transport
particles released from the water surface drop to deep
phase (passive particles), whose property is
water because of the violent mixing. Weak currents
unchanged and the change of the co-ordinate
below the water surface contribute little to the
depends on the velocity field. Thus, the fate of the
pollutant transport, which explains why there is no
tracers rests with the dynamic factors, such as the
obvious difference in the distribution of the
tide, wind and river runoff.
pollutants after 30 days between the experiments
with and without wind.
6.1 The influence of tide on pollutant transport
6.3 The influence of the river runoff on pollutant
The main difference between the experiments with
transport
and without tidal forcing (E1 and E2, E4 and E5) is
that the particles from bay head areas (S1, S2 and S4) Under the impact of the Coriolis force, most of the
without tidal forcing deflect to the west compared diluted water in the Changjiang River deflects south,
with the distribution with tidal forcing, because the enters Hangzhou Bay in the north and flows out of
tidal residual current direction in the inner bay is the bay in the south (Pan et al., 1997). This diluted
eastwards toward bay mouth (Liu et al., 2006). Zhu water becomes the main factor in driving the
(2000) also pointed out that the clockwise vortex in pollutant transport in the bay mouth area. So both in
the west was one of the main characteristics of the the wet and the dry seasons, without the Changjiang
residual current induced by the tide in the bay. This River runoff, particles released from the S3, S6 and
clockwise vortex in the west of Hangzhou Bay is S8 areas travel towards the north and enter the open
important to the mass transport; it brings the particles sea from the northeast of the bay. This phenomenon
in the bay head area and the middle of the bay to the is more obvious in the wet season. For example,
bay mouth. Therefore the tide is the main factor in particles released from S6 and S8 travel a longer
bringing the pollutants from the inner bay to the outer distance towards the north in E4 than in E8, and more
sea. In the bay mouth area, without the tidal forcing, particles from S3 in E4 escape beyond the numerical
the river runoff from the Changjiang River becomes boundary than in E8. Under the rush of the Qiantang
the main physical factor affecting the pollution River, most particles from the bay head area (S4 and
transport. The pollutants driven by this river flux S7) travel towards the east, so without this river
leave the bay from the south of the bay mouth very runoff, particles from S4 and S7 will go west, i.e.
quickly without tide-induced back-and-forth upstream.
movement. So it seems to be easier for the particles
7 CONCLUSIONS
in the bay mouth area to get out of the bay without
tidal forcing.
Based on the above analysis and discussion we
6.2 The influence of wind on the pollutant transport draw the following conclusions: (1) The tide and
Qiantang River discharge are the main factors to drive
Special events induced by strong wind such as
pollutants to leave bay head area. (2) The Changjiang River
storm surge are outside the scope of our study.
273
No.2 LI et al.: The impact of physical processes on pollutant transport in Hangzhou Bay
Fig.6 Particle distribution released from eight subdomains in first four trace experiment after 30 days
274 CHIN. J. OCEANOL. LIMNOL., 27(2), 2009 Vol.27
Fig.7 Particle distribution released from eight subdomains in last four trace experiment after 30 days
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8 ACKNOWLEDGEMENTS
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We gratefully acknowledge Mr. Sixun HUANG shallow bay. Environmental Pollution and Control 27(6):
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Lin, W.Q., S. Q. Lu and Y. Z. Chen, 2008. A study on the
suggestions, and Mr. Arthur Cracknell for his
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